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Article overview
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Impenetrable barriers in phase-space | S Wiggins
; L Wiesenfeld
; C Jaffé
; T Uzer
; | Date: |
11 Jun 2001 | Journal: | Phys Rev Lett, 86 (24), 5478-81 | Abstract: | Dynamical systems theory is used to construct a general phase-space version of transition state theory. Special multidimensional separatrices are found which act as impenetrable barriers in phase-space between reacting and nonreacting trajectories. The elusive momentum-dependent transition state between reactants and products is thereby characterized. A practical algorithm is presented and applied to a strongly coupled Hamiltonian. | Source: | PubMed, pmid11415280 | Services: | Forum | Review | Favorites |
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