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Charge-order-driven spin-peierls transition in alpha(')-NaxV2O5 | | Y Fagot-Revurat
; M Mehring
; R K Kremer
; | | Date: |
1 May 2000 | | Journal: | Phys Rev Lett, 84 (18), 4176-9 | | Abstract: | We conclude from 23Na and 51V NMR measurements in alpha(’)-NaxV2O5 (x = 0.996) (i) a charge-ordering transition starting at T</=37 K and preceding the lattice distortion and (ii) the formation of a spin gap Delta = 106 K at T(c) = 34.7 K. Above T(c), only a single Na site is observed in agreement with the Pmmn space group of this first 1/4-filled ladder system. Below T(c) = 34.7 K, this line evolves into eight distinct 23Na quadrupolar split lines, which evidences a lattice distortion with, at least, a doubling of the unit cell in the (a,b) plane. A model for this unique transition, implying both charge density wave and spin-Peierls order, is discussed. | | Source: | PubMed, pmid10990639 | | Services: | Forum | Review | Favorites | |
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