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18 April 2024
 
  » arxiv » 0907.3741

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Weak link behavior of grain boundaries in Co-doped BaFe2As2 pnictide superconductors
S. Lee ; J. Jiang ; J. D. Weiss ; C. M. Folkman ; C. W. Bark ; C. Tarantini ; A. Xu ; D. Abraimov ; A. Polyanskii ; C. T. Nelson ; Y. Zhang ; S. H. Baek ; H. W. Jang ; A. Yamamoto ; F. Kametani ; X. Q. Pan ; E. E. Hellstrom ; A. Gurevich ; C. B. Eom ; D. C. Larbalestier ;
Date 21 Jul 2009
AbstractThe discovery of any new high transition temperature Tc superconductor immediately poses the question of whether it has the essential qualities for applications: high critical current density Jc, high upper critical field Hc2 and irreversibility field Hirr, low anisotropy Hc2(ab)/Hc2(c) and capability of grain boundaries (GBs) to transmit supercurrent. YBa2Cu3O7-x fulfills all except the last requirement, resulting in more than 15 years of arduous development of sophisticated crystallographic texture fabrication processes to eliminate all but low angle GBs in useful conductor forms. In the recently discovered pnictide superconductors, novel Cooper pairing mediated by magnetic Fe ions leads to the second class of materials with Tc above 50 K. Here we show that despite their low anisotropy (<2), strong vortex pinning and high irreversibility field Hirr close to Hc2 which is well over 50 T, the critical current density Jb across [001] tilt GBs of thin film Ba(Fe1-xCox)2As2 bicrystals is strongly depressed, exhibiting weak link GB behavior similar to high-Tc cuprates. Our results suggest that weak-linked GBs are characteristic of high-Tc superconducting compounds with competing orders, low carrier density, and unconventional pairing symmetry and that GB properties require much greater attention if application hopes for high-Tc materials are to be fulfilled.
Source arXiv, 0907.3741
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