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Seebeck effect in Fe1+xTe1-ySey single crystals | I.Pallecchi
; G.Lamura
; M.Tropeano
; M.Putti
; R.Viennois
; E.Giannini
; D.Van der Marel
; | Date: |
1 Oct 2009 | Abstract: | We present measurements of resistivity and thermopower of Fe1+xTe1-ySey
single crystalline samples with y=0, 0.1, 0.2, 0.3 and 0.45 in zero field and
in a magnetic field B=8T. We propose a qualitative analysis of the temperature
behavior of S, where the samples are described as almost compensated
semimetals: different electron and hole bands with similar carrier
concentrations compete and their relative contribution to the thermoelectric
transport depends on the respective filling, mobility and coupling with
phonons. For y>=0.2, superconductivity occurs and the optimum Se-doping level
for a maximum Tc of 13 K turns out to be y=0.3. At low temperatures, evidence
of a contribution to S by an excitation-drag mechanism is found, while at high
temperatures a strikingly flat behavior of S is explained within a narrow band
Hubbard model. The support of a theoretical background which could provide band
resolved parameters such as carrier density, mobility and electron-phonon
coupling of each band would allow to extract from our data valuable
quantitative information on the transport and superconducting mechanisms of
these iron chalcogenides. | Source: | arXiv, 0910.0191 | Services: | Forum | Review | PDF | Favorites |
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