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28 March 2024
 
  » arxiv » 0912.2760

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Lowering of surface melting temperature in atomic clusters with a nearly closed shell structure
A. Bagrets ; R. Werner ; F. Evers ; G. Schneider ; D. Schooss ; P. Woelfle ;
Date 14 Dec 2009
AbstractWe investigate the interplay of particle number, N, and structural properties of selected clusters with N=12 up to N=562 by employing Gupta potentials parameterized for Aluminum and extensive Monte-Carlo simulations. Our analysis focuses on closed shell structures with extra atoms. The latter can put the cluster under a significant stress and we argue that typically such a strained system exhibits a reduced energy barrier for (surface) diffusion of cluster atoms. Consequently, also its surface melting temperature, T_S, is reduced, so that T_S separates from and actually falls well below the bulk value. The proposed mechanism may be responsible for the suppression of the surface melting temperature observed in a recent experiments.
Source arXiv, 0912.2760
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