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Geometry-controlled kinetics | O. Bénichou
; C. Chevalier
; J. Klafter
; B. Meyer
; R. Voituriez
; | Date: |
17 Jun 2010 | Abstract: | It has long been appreciated that transport properties can control reaction
kinetics. This effect can be characterized by the time it takes a diffusing
molecule to reach a target -- the first-passage time (FPT). Although essential
to quantify the kinetics of reactions on all time scales, determining the FPT
distribution was deemed so far intractable. Here, we calculate analytically
this FPT distribution and show that transport processes as various as regular
diffusion, anomalous diffusion, diffusion in disordered media and in fractals
fall into the same universality classes. Beyond this theoretical aspect, this
result changes the views on standard reaction kinetics. More precisely, we
argue that geometry can become a key parameter so far ignored in this context,
and introduce the concept of "geometry-controlled kinetics". These findings
could help understand the crucial role of spatial organization of genes in
transcription kinetics, and more generally the impact of geometry on
diffusion-limited reactions. | Source: | arXiv, 1006.3477 | Services: | Forum | Review | PDF | Favorites |
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