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23 April 2024
 
  » arxiv » 1103.1039

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Low-moment magnetism in the double perovskites Ba2MOsO6 (M=Li,Na)
Andrew J. Steele ; Peter J. Baker ; Tom Lancaster ; Francis L. Pratt ; Isabel Franke ; Saman Ghannadzadeh ; Paul A. Goddard ; William Hayes ; D. Prabhakaran ; Stephen J. Blundell ;
Date 5 Mar 2011
AbstractThe magnetic ground states of the isostructural double perovskites Ba$_2$NaOsO$_6$ and Ba$_2$LiOsO$_6$ are investigated with muon-spin rotation. In Ba$_2$NaOsO$_6$ long-range magnetic order is detected via the onset of a spontaneous muon-spin precession signal below $T_{mathrm{c}}=7.2pm 0.2;mathrm{K}$, while in Ba$_2$LiOsO$_6$ a static but spatially-disordered internal field is found below 8 K. A novel probabilistic argument is used to show from the observed precession frequencies that the magnetic ground state in Ba$_2$NaOsO$_6$ is most likely to be low-moment ($approx 0.2$,$mu_{ m B}$) ferromagnetism and not canted antiferromagnetism. Ba$_2$LiOsO$_6$ is antiferromagnetic and we find a spin-flop transition at 5.5,T. A reduced osmium moment is common to both compounds, probably arising from a combination of spin-orbit coupling and frustration.
Source arXiv, 1103.1039
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