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25 April 2024
 
  » arxiv » 1111.0817

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Fermi Level Tuning of Epitaxial Sb2Te3 Thin Films on Graphene by Regulating Intrinsic Defects and Substrate Transfer Doping
Yeping Jiang ; Y. Y. Sun ; Mu Chen ; Yilin Wang ; Zhi Li ; Canli Song ; Ke He ; Lili Wang ; Xi Chen ; Qi-Kun Xue ; Xucun Ma ; S. B. Zhang ;
Date 3 Nov 2011
AbstractHigh-quality Sb2Te3 films are obtained by molecular beam epitaxy on graphene substrate and investigated by in situ scanning tunneling microscopy/spectroscopy. Intrinsic defects responsible for the natural p-type conductivity of Sb2Te3 are identified to be the Sb vacancies and SbTe antisites in agreement with first-principles calculations. By minimizing defect densities, coupled with a transfer doping by the graphene substrate, the Fermi level of Sb2Te3 thin films can be tuned over the entire range of the bulk band gap. This establishes the necessary condition to explore topological insulator behaviors near the Dirac point.
Source arXiv, 1111.0817
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