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19 April 2024

» arxiv » 1209.3181

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Formation and relaxation of RbHe exciplexes on He nanodroplets studied by femtosecond pump and picosecond probe spectroscopy
C. Giese ; T. Mullins ; B. Gruener ; M. Weidemueller ; F. Stienkemeier ; M. Mudrich ;
Date:	14 Sep 2012
Abstract:	Vibrationally resolved photoionization spectra of RbHe exciplexes forming on He nanodroplets are recorded using femtosecond pump-probe spectroscopy with amplitude-shaped probe pulses. The time-evolution of the spectra reveals an exciplex formation time ~10ps followed by vibrational relaxation extending up to >1ns. This points to an indirect, time-delayed desorption process of RbHe off the He surface.
Source:	arXiv, 1209.3181
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