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25 April 2024
 
  » arxiv » 1303.3308

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A Ni-Fe Layered Double Hydroxide-Carbon Nanotube Complex for Water Oxidation
Ming Gong ; Yanguang Li ; Hailiang Wang ; Yongye Liang ; Justin Zachary Wu ; Jigang Zhou ; Jian Wang ; Tom Regier ; Fei Wei ; Hongjie Dai ;
Date 14 Mar 2013
AbstractHighly active, durable and cost-effective electrocatalysts for water oxidation to evolve oxygen gas hold a key to a range of renewable energy solutions including water splitting and rechargeable metal-air batteries. Here, we report the synthesis of ultrathin nickel iron layered double hydroxide nanoplates on mildly oxidized multi-walled carbon nanotubes. Incorporation of Fe into the nickel hydroxide induced the formation of NiFe-layered double hydroxide. The nanoplates were covalently attached to a network of nanotubes, affording excellent electrical wiring to the nanoplates. The ultra-thin Ni-Fe layered double hydroxide nanoplates/carbon nanotube complex was found to exhibit unusually high electro-catalytic activity and stability for oxygen evolution and outperformed commercial precious metal Ir catalysts.
Source arXiv, 1303.3308
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