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20 April 2024
 
  » arxiv » 1308.0185

 Article overview


Electronic superlattice revealed by resonant scattering from random impurities in Sr3Ru2O7
M.A. Hossain ; I. Zegkinoglou ; Y.-D. Chuang ; J. Geck ; B. Bohnenbuck ; A.G. Cruz Gonzalez ; H.-H. Wu ; C. Schussler-Langeheine ; D.G. Hawthorn ; J.D. Denlinger ; R. Mathieu ; Y. Tokura ; S. Satow ; H. Takagi ; Y. Yoshida ; Z. Hussain ; B. Keimer ; G.A. Sawatzky ; A. Damascelli ;
Date 1 Aug 2013
AbstractResonant elastic x-ray scattering (REXS) is an exquisite element-sensitive tool for the study of subtle charge, orbital, and spin superlattice orders driven by the valence electrons, which therefore escape detection in conventional x-ray diffraction (XRD). Although the power of REXS has been demonstrated by numerous studies of complex oxides performed in the soft x-ray regime, the cross section and photon wavelength of the material-specific elemental absorption edges ultimately set the limit to the smallest superlattice amplitude and periodicity one can probe. Here we show -- with simulations and REXS on Mn-substituted Sr$_3$Ru$_2$O$_7$ -- that these limitations can be overcome by performing resonant scattering experiments at the absorption edge of a suitably-chosen, dilute impurity. This establishes that -- in analogy with impurity-based methods used in electron-spin-resonance, nuclear-magnetic resonance, and M"ossbauer spectroscopy -- randomly distributed impurities can serve as a non-invasive, but now momentum-dependent probe, greatly extending the applicability of resonant x-ray scattering techniques.
Source arXiv, 1308.0185
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