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24 April 2024
 
  » arxiv » cond-mat/0308482

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Optical spectra of quantum dots: effects of non-adiabaticity
J. T. Devreese ; V. M. Fomin ; E. P. Pokatilov ; V. N. Gladilin ; S. N. Klimin ;
Date 25 Aug 2003
Journal Phys. Stat. Sol. (c) 0 (2003) 1189
Subject Mesoscopic Systems and Quantum Hall Effect | cond-mat.mes-hall
Affiliation1,2), E. P. Pokatilov , V. N. Gladilin (1,2), S. N. Klimin (1,2) ( TFVS, Universiteit Antwerpen - UIA, FSM, Universitatea de Stat din Moldova
AbstractIt is shown that in many cases an adequate description of optical spectra of semiconductor quantum dots requires a treatment beyond the commonly used adiabatic approximation. We have developed a theory of phonon-assisted optical transitions in semiconductor quantum dots, which takes into account non-adiabaticity of the exciton-phonon system. Effects of non-adiabaticity lead to a mixing of different exciton and phonon states that provides a key to the understanding of surprisingly high intensities of phonon satellites observed in photoluminescence spectra of quantum dots. A breakdown of the adiabatic approximation gives an explanation also for discrepancies between the serial law, observed in multi-phonon optical spectra of some quantum dots, and the Franck-Condon progression, prescribed by the adiabatic approach.
Source arXiv, cond-mat/0308482
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