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19 April 2024
 
  » arxiv » 1504.0309

 Article overview


Ferroelectric Skyrmions and a Zoo of Multiferroic Phases in GaV4S8
E. Ruff ; S. Widmann ; P. Lunkenheimer ; V. Tsurkan ; S. Bordács ; I. Kézsmárki ; A. Loidl ;
Date 1 Apr 2015
AbstractThe lacunar spinel GaV4S8 undergoes orbital ordering at 44 K and reveals a complex magnetic phase diagram below 13 K, including a ferromagnetic, cycloidal and N’eel-type skyrmion lattice phase. Skyrmions are topologically protected nano-scale spin vortices with fascinating physical properties and high potential for future data storage. Here we provide a detailed study of the polar properties of GaV4S8, revealing that its orbitally ordered phase is ferroelectric with sizable polarization of ~ 1 {mu}C/cm^2. Moreover, spin-driven excess polarizations emerge in all magnetic phases, hence, GaV4S8 hosts three different multiferroic phases including the skyrmion lattice formed by ferroelectric spin vortices. By taking into account the crystal symmetry and spin patterns of the magnetically ordered phases, exchange striction is identified as the main microscopic mechanism behind the spin-driven ferroelectric polarization in each multiferroic phase. The polar crystal structure of GaV4S8 is unique among the known skyrmion-lattice host materials and the ferroelectric SkL phase may be exploited for non-dissipative electric-field control of skyrmions.
Source arXiv, 1504.0309
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