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25 April 2024
 
  » arxiv » 1511.3573

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Point-to-set lengths, local structure, and glassiness
Sho Yaida ; Ludovic Berthier ; Patrick Charbonneau ; Gilles Tarjus ;
Date 11 Nov 2015
AbstractThe growing sluggishness of glass-forming liquids is thought to be accompanied by growing structural order. The nature of such order, however, remains hotly debated. A decade ago, point-to-set (PTS) correlation lengths were proposed as measures of amorphous order in glass formers, but recent results raise doubts as to their generality. Here, we extend the definition of PTS correlations in order to agnostically capture any type of growing order in liquids, be it local or amorphous. This advance clarifies the nature of PTS correlations, and enables the formulation of a clear distinction between slowing down due to conventional critical ordering from that due to glassiness.
Source arXiv, 1511.3573
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