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20 April 2024
 
  » arxiv » 1607.2271

 Article overview


Rearrangement zone around a crack tip in a double self-assembled transient network
Guillaume Foyart ; Christian Ligoure ; Serge Mora ; Laurence Ramos ;
Date 8 Jul 2016
AbstractWe investigate the nucleation and propagation of cracks in self-assembled viscoelastic fluids, which are made of surfactant micelles reversibly linked by telechelic polymers. The morphology of the micelles can be continuously tuned, from spherical to rod-like to wormlike, thus producing transient double networks when the micelles are sufficiently long and entangled, and transient single networks otherwise. For a single network, we show that cracks nucleate when the sample deformation rate involved is comparable to the relaxation time scale of the network. For a double network, by contrast, significant rearrangements of the micelles occur as a crack nucleates and propagates. We show that birefringence develops at the crack tip over a finite length, $xi$, which corresponds to the length scale over which micelles alignment occur. We find that $xi$ is larger for slower cracks, suggesting an increase of ductility.
Source arXiv, 1607.2271
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