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23 April 2024
 
  » arxiv » 1612.4863

 Article overview


Directional Interlayer Spin-Valley Transfer in Two-Dimensional Heterostructures
John R. Schaibley ; Pasqual Rivera ; Hongyi Yu ; Kyle L. Seyler ; Jiaqiang Yan ; David G. Mandrus ; Takashi Taniguchi ; Kenji Watanabe ; Wang Yao ; Xiaodong Xu ;
Date 14 Dec 2016
AbstractVan der Waals heterostructures formed by two different monolayer semiconductors have emerged as a promising platform for new optoelectronic and spin/valleytronic applications. In addition to its atomically thin nature, a two-dimensional semiconductor heterostructure is distinct from its three-dimensional counterparts due to the unique coupled spin-valley physics of its constituent monolayers. Here, we report the direct observation that an optically generated spin-valley polarization in one monolayer can be transferred between layers of a two-dimensional MoSe2-WSe2 heterostructure. Using nondegenerate optical circular dichroism spectroscopy, we show that charge transfer between two monolayers conserves spin-valley polarization and is only weakly dependent on the twist angle between layers. Our work points to a new spin-valley pumping scheme in nanoscale devices, provides a fundamental understanding of spin-valley transfer across the two-dimensional interface, and shows the potential use of two-dimensional semiconductors as a spin-valley generator in 2D spin/valleytronic devices for storing and processing information.
Source arXiv, 1612.4863
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