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23 April 2024
 
  » arxiv » 1612.7444

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Nonlinear photoluminescence imaging of isotropic and liquid crystalline dispersions of graphene oxide
Bohdan Senyuk ; Natnael Behabtu ; Benjamin G. Pacheco ; Taewoo Lee ; Gabriel Ceriotti ; James M. Tour ; Matteo Pasquali ; Ivan I. Smalyukh ;
Date 22 Dec 2016
AbstractWe report a visible-range nonlinear photoluminescence (PL) from graphene oxide (GO) flakes excited by near-infrared femtosecond laser light. PL intensity has nonlinear dependence on the laser power, implying a multiphoton excitation process, and also strongly depends on a linear polarization orientation of excitation light, being at maximum when it is parallel to flakes. We show that PL can be used for a fully three-dimensional label-free imaging of isotropic, nematic, and lamellar liquid crystalline dispersions of GO flakes in water. This nonlinear PL is of interest for applications in direct label-free imaging of composite materials and study of orientational ordering in mesomorphic phases formed by these flakes, as well as in biomedical and sensing applications utilizing GO.
Source arXiv, 1612.7444
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