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Stacking order dynamic in the quasi-two-dimensional dichalcogenide 1T-TaS$_2$ probed with MeV ultrafast electron diffraction | L. Le Guyader
; T. Chase
; A. Reid
; R.K. Li
; D. Svetin
; X. Shen
; T. Vecchione
; X.J. Wang
; D. Mihailovic
; H.A. Dürr
; | Date: |
15 Mar 2017 | Abstract: | Transitions between different charge density wave (CDW) states in
quasi-two-dimensional materials may be accompanied also by changes in the
inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the
out-of-plane stacking order dynamics in the quasi-two-dimensional
dichalcogenide 1T-TaS$_2$ is investigated for the first time. From the
intensity of the CDW satellites aligned around the commensurate $l$ = 1/6
characteristic stacking order, it is found out that this phase disappears with
a 0.5 ps time constant. Simultaneously, in the same experiment, the emergence
of the incommensurate phase, with a slightly slower 2.0 ps time constant, is
determined from the intensity of the CDW satellites aligned around the
incommensurate $l$ = 1/3 characteristic stacking order. These results might be
of relevance in understanding the metallic character of the laser-induced
metastable "hidden" state recently discovered in this compound. | Source: | arXiv, 1703.5035 | Services: | Forum | Review | PDF | Favorites |
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