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26 April 2024
 
  » arxiv » 1703.5035

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Stacking order dynamic in the quasi-two-dimensional dichalcogenide 1T-TaS$_2$ probed with MeV ultrafast electron diffraction
L. Le Guyader ; T. Chase ; A. Reid ; R.K. Li ; D. Svetin ; X. Shen ; T. Vecchione ; X.J. Wang ; D. Mihailovic ; H.A. Dürr ;
Date 15 Mar 2017
AbstractTransitions between different charge density wave (CDW) states in quasi-two-dimensional materials may be accompanied also by changes in the inter-layer stacking of the CDW. Using MeV ultrafast electron diffraction, the out-of-plane stacking order dynamics in the quasi-two-dimensional dichalcogenide 1T-TaS$_2$ is investigated for the first time. From the intensity of the CDW satellites aligned around the commensurate $l$ = 1/6 characteristic stacking order, it is found out that this phase disappears with a 0.5 ps time constant. Simultaneously, in the same experiment, the emergence of the incommensurate phase, with a slightly slower 2.0 ps time constant, is determined from the intensity of the CDW satellites aligned around the incommensurate $l$ = 1/3 characteristic stacking order. These results might be of relevance in understanding the metallic character of the laser-induced metastable "hidden" state recently discovered in this compound.
Source arXiv, 1703.5035
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