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25 April 2024
 
  » arxiv » 1703.8248

 Article overview



Molecular quantum spin network controlled by a single qubit
Lukas Schlipf ; Thomas Oeckinghaus ; Kebiao Xu ; Durga Bhaktavatsala Rao Dasari ; Andrea Zappe ; Felipe Fávaro de Oliveira ; Bastian Kern ; Mykhailo Azarkh ; Malte Drescher ; Markus Ternes ; Klaus Kern ; Jörg Wrachtup ; Amit Finkler ;
Date 23 Mar 2017
AbstractScalable quantum technologies will require an unprecedented combination of precision and complexity for designing stable structures of well-controllable quantum systems. It is a challenging task to find a suitable elementary building block, of which a quantum network can be comprised in a scalable way. Here we present the working principle of such a basic unit, engineered using molecular chemistry, whose control and readout are executed using a nitrogen vacancy (NV) center in diamond. The basic unit we investigate is a synthetic polyproline with electron spins localized on attached molecular sidegroups separated by a few nanometers. We demonstrate the readout and coherent manipulation of very few ($leq 6 $) of these $S=1/2$ electronic spin systems and access their direct dipolar coupling tensor. Our results show, that it is feasible to use spin-labeled peptides as a resource for a molecular-qubit based network, while at the same time providing simple optical readout of single quantum states through NV-magnetometry. This work lays the foundation for building arbitrary quantum networks using well-established chemistry methods, which has many applications ranging from mapping distances in single molecules to quantum information processing.
Source arXiv, 1703.8248
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