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24 April 2024
 
  » arxiv » 1907.3839

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Coexisting spin resonance and long-range magnetic order of Eu in EuRbFe$_4$As$_4$
K. Iida ; Y. Nagai ; S. Ishida ; M. Ishikado ; N. Murai ; A. D. Christianson ; H. Yoshida ; Y. Inamura ; H. Nakamura ; A. Nakao ; K. Munakata ; D. Kagerbauer ; M. Eisterer ; K. Kawashima ; Y. Yoshida ; H. Eisaki ; A. Iyo ;
Date 8 Jul 2019
AbstractMagnetic excitations and magnetic structure of EuRbFe$_4$As$_4$ were investigated by inelastic neutron scattering (INS), neutron diffraction, and random phase approximation (RPA) calculations. Below the superconducting transition temperature $T_ ext{c}=36.5$~K, the INS spectra exhibit the neutron spin resonances at $Q_ ext{res}=1.27(2)$~$ ext{AA}^{-1}$ and $1.79(3)$~$ ext{AA}^{-1}$. They correspond to the $mathbf{Q}=(0.5,0.5,1)$ and $(0.5,0.5,3)$ nesting wave vectors, showing three dimensional nature of the band structure. The characteristic energy of the neutron spin resonance is $E_ ext{res}=17.7(3)$~meV corresponding to $5.7(1)k_ ext{B}T_ ext{c}$. Observation of the neutron spin resonance mode and our RPA calculations in conjunction with the recent optical conductivity measurements are indicative of the $s_pm$ superconducting pairing symmetry in EuRbFe$_4$As$_4$. In addition to the neutron spin resonance mode, upon decreasing temperature below the magnetic transition temperature $T_ ext{N}=15$~K, the spin wave excitation originating in the long-range magnetic order of the Eu sublattice was observed in the low-energy inelastic channel. Single-crystal neutron diffraction measurements demonstrate that the magnetic propagation vector of the Eu sublattice is $mathbf{k}=(0, 0, 0.25)$, representing the three-dimensional antiferromagnetic order. Linear spin wave calculations assuming the obtained magnetic structure with the intra- and inter-plane nearest neighbor exchange couplings of $J_1/k_ ext{B}=-1.31$~K and $J_c/k_ ext{B}=0.08$~K can reproduce quantitatively the observed spin wave excitation. Our results show that superconductivity and long-range magnetic order of Eu coexist in EuRbFe$_4$As$_4$ whereas the coupling between them is rather weak.
Source arXiv, 1907.3839
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