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23 April 2024 |
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Spin entropy as the likely source of enhanced thermopower in $
mf Na_xCo_2O_4 | Yayu Wang
; Nyrissa S. Rogado
; R. J. Cava
; N. P. Ong
; | Date: |
4 Jun 2004 | Journal: | Nature 423, 425 (2003) | Subject: | Strongly Correlated Electrons; Materials Science | cond-mat.str-el cond-mat.mtrl-sci | Abstract: | In an electric field, the flow of electrons in a solid produces an entropy current in addition to the familiar charge current. This Peltier effect underlies all thermoelectric refrigerators. The upsurge in thermoelectric cooling applications has led to a search for more efficient Peltier materials and to renewed theoretical interest in how electron-electron interaction may enhance the thermopower $Q$ of materials such as the transition-metal oxides cite{Mahan,Beni,Kotliar,Chaikin}. An important factor in this enhancement is the electronic spin entropy, which is predicted cite{Chaikin,Kwak,KwakChaikin} to dominate the entropy current. Here we report evidence for such suppression in the layered oxide $
m Na_xCo_2O_4$, and present evidence that it is a strong-correlation effect. | Source: | arXiv, cond-mat/0406125 | Services: | Forum | Review | PDF | Favorites |
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