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Strongly correlated properties of the thermoelectric cobalt oxide Ca3Co4O9 | P. Limelette
; V. Hardy
; P. Auban-Senzier
; D. Jerome
; D. Flahaut
; S. Hebert
; R. Fresard
; Ch. Simon
; J. Noudem
; A. Maignan
; | Date: |
19 May 2005 | Journal: | Phys. Rev. B. 71, 233108 (2005) DOI: 10.1103/PhysRevB.71.233108 | Subject: | Strongly Correlated Electrons; Materials Science | cond-mat.str-el cond-mat.mtrl-sci | Abstract: | We have performed both in-plane resistivity, Hall effect and specific heat measurements on the thermoelectric cobalt oxide Ca$_{3}$Co$_{4}$O$_{9}$. Four distinct transport regimes are found as a function of temperature, corresponding to a low temperature insulating one up to $T_{min}approx $63 K, a strongly correlated Fermi liquid up to $T^*approx $140 K, with $
ho=
ho_0+AT^2$ and $Aapprox 3.63$ $10^{-2} mu Omega cm/K^{2}$, followed by an incoherent metal with $k_Flleq 1$ and a high temperature insulator above T$^{**}approx $510 K . Specific heat Sommerfeld coefficient $gamma = 93$ mJ/(mol.K$^{2}$) confirms a rather large value of the electronic effective mass and fulfils the Kadowaki-Woods ratio $A/gamma^2 approx 0.45$ 10$^{-5}$ $mu Omega cm.K^2/(mJ^2mol^{-2})$. Resistivity measurements under pressure reveal a decrease of the Fermi liquid transport coefficient A with an increase of $T^*$ as a function of pressure while the product $A(T^*)^2/a$ remains constant and of order $h/e^2$. Both thermodynamic and transport properties suggest a strong renormalization of the quasiparticles coherence scale of order $T^*$ that seems to govern also thermopower. | Source: | arXiv, cond-mat/0505464 | Services: | Forum | Review | PDF | Favorites |
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