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Orientation and Motion of Water Molecules at Air/Water Interface | | Wei Gan
; Dan Wu
; Zhen Zhang
; Hong-fei Wang
; | | Date: |
22 Aug 2005 | | Subject: | Other | cond-mat.other | | Abstract: | Analysis of SFG vibrational spectra of OH stretching bands in four experimental configurations shows that orientational motion of water molecule at air/water interface is libratory within a limited angular range. This picture is significantly different from the previous conclusion that the interfacial water molecule orientation varies over a broad range within the vibrational relaxation time, the only direct experimental evidence for ultrafast and broad orientational motion of a liquid interface by Wei et al. [Phys. Rev. Lett. 86, 4799, (2001)] using single SFG experimental configuration. | | Source: | arXiv, cond-mat/0508525 | | Services: | Forum | Review | PDF | Favorites | |
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