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Interplay of creation, propagation, and relaxation of an excitation in a dimer | | J. Perina
; Jr.
; | | Date: |
6 Dec 1998 | | Journal: | Chem.Phys. 236 (1998) 157-179 | | Subject: | quant-ph | | Affiliation: | Institute of Physics of Charles University | | Abstract: | Interplay of simultaneous creation, annihilation, propagation, and relaxation of an excitation in molecular condensates interacting with an ultrashort quantum optical pulse is studied in general and specialized to a dimer. A microscopic model appropriate for such systems (with strong exciton-phonon coupling) is presented. It also incorporates effects of (quantum) noise in the optical field. A variety of new features in the initial stage of excitation dynamics (when it is being created) is revealed; a strong influence of the coherent excitation propagation on the processes of excitation creation and annihilation in a molecule strongly interacting with phonons is the most remarkable one. | | Source: | arXiv, quant-ph/9901007 | | Services: | Forum | Review | PDF | Favorites | |
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