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Fluid-solid phase-separation in hard-sphere mixtures is unrelated to bond-percolation | | A. A. Louis
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18 Dec 1999 | | Journal: | Phys. Rev. Lett. 84, 1840 (2000) | | Subject: | Soft Condensed Matter; Statistical Mechanics | cond-mat.soft cond-mat.stat-mech | | Affiliation: | Dept. of Chemistry, Cambridge University | | Abstract: | In a recent letter, Buhot proposes that entropy driven phase-separation in hard-core binary mixtures is directly related to a bond-percolation transition. However, at least for binary hard-sphere mixtures, calculations based on an accurate approximation to g_{ll}(r) demonstrate that n_b varies widely along the phase-boundaries calculated directly by simulations, implying that bond-percolation is unrelated to the phase-separation in these systems. | | Source: | arXiv, cond-mat/0001241 | | Services: | Forum | Review | PDF | Favorites | |
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