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05 November 2024
 
  » arxiv » cond-mat/9307007

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Nonlinear Optical Response of C60 Molecules
Kikuo Harigaya ; Shuji Abe ;
Date 6 Jul 1993
Journal J. Luminescence 60&61 (1994) 380-382 DOI: 10.1016/0022-2313(94)90170-8
Subject cond-mat
Affiliation1,2) and Shuji Abe , ( Elecrotechnical Laboratory, Umezono, Tsukuba, Ibaraki, Japan, Department of Physics, University of Sheffield, United Kingdom
AbstractThe third-order nonlinear optical susceptiblity chi(3) of a C60 molecule is calculated by using a free-electron model as well as by taking Coulomb interactions into account. The free-electron model yields chi(3) magnitudes which are in agreement with experiment. Althugh Coulomb interactions reduce chi(3) by one order of magnitude, local-field corrections can be invoked to recover the agreement.
Source arXiv, cond-mat/9307007
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