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26 April 2024
 
  » arxiv » cond-mat/0108130

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Magnetic Excitations of the Spin Gap System TlCuCl$_3$
A. Oosawa ; T. Kato ; H. Tanaka ; K. Kakurai ; M. Mueller ; H. -J. Mikeska ;
Date 8 Aug 2001
Subject Strongly Correlated Electrons | cond-mat.str-el
AbstractTlCuCl$_3$ has a singlet ground state with the excitation gap $Delta =0.65$ meV. The magnetic excitations in TlCuCl$_3$ have been investigated by means of neutron inelastic scattering experiments. The constant-$it{pmb Q}$ energy scan profiles were collected in the $a^*-c^*$ plane. A well-defined single magnetic excitation mode was observed. The dispersion relations along four different directions were determined. The lowest excitation occurs at ${it{pmb Q}}=(h, 0, l)$ with integer $h$ and odd $l$, as observed in KCuCl$_3$. A cluster series expansion up to the sixth order was applied to analyze the dispersion relations, and the individual exchange interactions were evaluated. It was demonstrated that TlCuCl$_3$ is a strongly coupled spin-dimer system.
Source arXiv, cond-mat/0108130
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