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Imaging and control of interfering wave packets in a dissociating molecule | | Esben Skovsen
; Mette Machholm
; Tine Ejdrup
; Jan Thøgersen
; Henrik Stapelfeldt
; | | Date: |
23 Sep 2002 | | Journal: | Phys Rev Lett, 89 (13), 133004 | | Abstract: | Using two identical 110 femtosecond (fs) optical pulses separated by 310 fs, we launch two dissociative wave packets in I2. We measure the square of the wave function as a function of both the internuclear separation, /Psi(R)/(2), and of the internuclear velocity, /Psi(v(R))/(2), by ionizing the dissociating molecule with an intense 20 fs probe pulse. Strong interference is observed in both /Psi(R)/(2) and in /Psi(v(R))/(2). The interference, and therefore the shape of the wave function, is controlled through the phase difference between the two dissociation pulses in good agreement with calculations. | | Source: | PubMed, pmid12225023 | | Services: | Forum | Review | Favorites | |
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