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26 April 2024
 
  » arxiv » 0912.4376

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NMR study of the high-field magnetic phase of LiCuVO$_4$
N. Buttgen ; W. Kraetschmer ; L.E. Svistov ; L.A. Prozorova ; A. Prokofiev ;
Date 22 Dec 2009
AbstractWe report on NMR studies of the quasi--1D antiferromagnetic $S=1/2$ chain cuprate LiCuVO$_4$, focusing on the high--field spin--modulated phase observed recently in applied magnetic fields $H > H_{ m c2}$ ($mu_0H_{ m c2} approx 7.5$ T). The NMR spectra of $^7$Li and $^{51}$V around the transition from the ordered to the paramagnetic state were measured. It is shown that the spin--modulated magnetic structure forms with ferromagnetic interactions between spins of neighboring chains within the {f ab}--plane at low temperatures 0.6 K $ < T < T_{ m N}$. The best fit provides evidence that the mutual orientation between spins of neighboring {f ab}--planes is random. For elevated temperatures $T_{ m N} < T lesssim 15$ K, short--range magnetic order occurs at least on the characteristic time scale of the NMR experiment.
Source arXiv, 0912.4376
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