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26 April 2024
 
  » arxiv » 1305.5426

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Observation of antiferromagnetic order collapse in the pressurized insulator LaMnPO
Jing Guo ; J. W. Simonson ; Liling Sun ; Qi Wu ; Peiwen Gao ; Chao Zhang ; Dachun Gu ; Gabriel Kotliar ; Meigan Aronson ; Zhongxian Zhao ;
Date 23 May 2013
AbstractThe emergence of superconductivity in the iron pnictide and cuprate high temperature superconductors usually accompanies the suppression of an antiferromagnetically (AFM) ordered state in a corresponding parent compound through the use of chemical doping or external pressure1-5. A great deal of effort has been made to find superconductivity in Mn-based compounds6-14, which are thought to bridge the gap between the two families of high temperature superconductors7,15,16, but long-ranged AFM order was not successfully suppressed via chemical doping in these investigations. Here we report the first observation of the pressure-induced elimination of long-ranged AFM order in LaMnPO single crystals that are iso-structural to the LaFeAsO superconductor15,17. By combining in-situ high pressure resistance and ac susceptibility measurements, we found that LaMnPO undergoes a crossover from an AFM insulating to an AFM metallic state at a pressure ~20 GPa and that the long-ranged AFM order collapses at a higher pressure ~32 GPa. Our findings are of importance to explore potential superconductivity in Mn-based compounds and to shed new light on the underlying mechanism of high temperature superconductivity.
Source arXiv, 1305.5426
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