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26 April 2024
 
  » arxiv » cond-mat/0306054

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Signatures of valence fluctuations in CeCu2Si2 under high pressure
A. T. Holmes ; D. Jaccard ; K. Miyake ;
Date 3 Jun 2003
Journal Phys. Rev. B 69, 024508 (2004) DOI: 10.1103/PhysRevB.69.024508
Subject Strongly Correlated Electrons; Superconductivity | cond-mat.str-el cond-mat.supr-con
Affiliation University of Geneva, Switzerland, University of Osaka, Japan
AbstractSimultaneous resistivity and a.c.-specific heat measurements have been performed under pressure on single crystalline CeCu2Si2 to over 6 GPa in a hydrostatic helium pressure medium. A series of anomalies were observed around the pressure coinciding with a maximum in the superconducting critical temperature, $T_c^{max}$. These anomalies can be linked with an abrupt change of the Ce valence, and suggest a second quantum critical point at a pressure $P_v simeq 4.5$ GPa, where critical valence fluctuations provide the superconducting pairing mechanism, as opposed to spin fluctuations at ambient pressure. Such a valence instability, and associated superconductivity, is predicted by an extended Anderson lattice model with Coulomb repulsion between the conduction and f-electrons. We explain the T-linear resistivity found at $P_v$ in this picture, while other anomalies found around $P_v$ can be qualitatively understood using the same model.
Source arXiv, cond-mat/0306054
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