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27 April 2024

» arxiv » 1601.7481

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On the bonding environment of phosphorus in purified doped single-walled carbon nanotubes
Georgina Ruiz-Soria ; Toma Susi ; Markus Sauer ; Kazuhiro Yanagi ; Thomas Pichler ; Paola Ayala ;
Date:	27 Jan 2016
Abstract:	In this work, phosphorous-doped single-walled carbon nanotubes have been synthesized by the thermal decomposition of trimethylphosphine using a high-vacuum chemical vapor deposition method. Furthermore, a modified density-gradient-ultracentrifugation process has been applied to carefully purify our doped material. The combined use of Raman and X-ray photoelectron spectroscopy allowed us to provide the first insight into the bonding environment of P incorporated into the carbon lattice, avoiding competing signals arising from synthesis byproducts. This study represents the first step toward the identification of the bonding configuration of P atoms when direct substitution takes place.
Source:	arXiv, 1601.7481
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