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27 April 2024
 
  » arxiv » cond-mat/0401190

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Lattice theory of trapping reactions with mobile species
M.Moreau ; G.Oshanin ; O.Benichou ; M.Coppey ;
Date 12 Dec 2003
Subject Statistical Mechanics | cond-mat.stat-mech
Affiliation LPTL, University of Paris 6, Paris, France; LPMC, College de France, Paris, France
AbstractWe present a stochastic lattice theory describing the kinetic behavior of trapping reactions $A + B o B$, in which both the $A$ and $B$ particles perform an independent stochastic motion on a regular hypercubic lattice. Upon an encounter of an $A$ particle with any of the $B$ particles, $A$ is annihilated with a finite probability; finite reaction rate is taken into account by introducing a set of two-state random variables - "gates", imposed on each $B$ particle, such that an open (closed) gate corresponds to a reactive (passive) state. We evaluate here a formal expression describing the time evolution of the $A$ particle survival probability, which generalizes our previous results. We prove that for quite a general class of random motion of the species involved in the reaction process, for infinite or finite number of traps, and for any time $t$, the $A$ particle survival probability is always larger in case when $A$ stays immobile, than in situations when it moves.
Source arXiv, cond-mat/0401190
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